在这个论坛上，将“乔什”归功。

Application.Quit()并且Process.Kill()是可能的解决方案，但已证明是不可靠的。当主应用程序死亡时，您仍然可以运行子进程。我们真正想要的是子进程在主进程死亡后立即死亡。

解决方案是使用“作业对象” http://msdn.microsoft.com/zh-
cn/library/ms682409(VS.85).aspx。

这个想法是为您的主应用程序创建一个“作业对象”，并向该作业对象注册子进程。如果主进程终止，则操作系统将负责终止子进程。

public enum JobObjectInfoType
{
    AssociateCompletionPortInformation = 7,
    BasicLimitInformation = 2,
    BasicUIRestrictions = 4,
    EndOfJobTimeInformation = 6,
    ExtendedLimitInformation = 9,
    SecurityLimitInformation = 5,
    GroupInformation = 11
}

[StructLayout(LayoutKind.Sequential)]
public struct SECURITY_ATTRIBUTES
{
    public int nLength;
    public IntPtr lpSecurityDescriptor;
    public int bInheritHandle;
}

[StructLayout(LayoutKind.Sequential)]
struct JOBOBJECT_BASIC_LIMIT_INFORMATION
{
    public Int64 PerProcessUserTimeLimit;
    public Int64 PerJobUserTimeLimit;
    public Int16 LimitFlags;
    public UInt32 MinimumWorkingSetSize;
    public UInt32 MaximumWorkingSetSize;
    public Int16 ActiveProcessLimit;
    public Int64 Affinity;
    public Int16 PriorityClass;
    public Int16 SchedulingClass;
}

[StructLayout(LayoutKind.Sequential)]
struct IO_COUNTERS
{
    public UInt64 ReadOperationCount;
    public UInt64 WriteOperationCount;
    public UInt64 OtherOperationCount;
    public UInt64 ReadTransferCount;
    public UInt64 WriteTransferCount;
    public UInt64 OtherTransferCount;
}

[StructLayout(LayoutKind.Sequential)]
struct JOBOBJECT_EXTENDED_LIMIT_INFORMATION
{
    public JOBOBJECT_BASIC_LIMIT_INFORMATION BasicLimitInformation;
    public IO_COUNTERS IoInfo;
    public UInt32 ProcessMemoryLimit;
    public UInt32 JobMemoryLimit;
    public UInt32 PeakProcessMemoryUsed;
    public UInt32 PeakJobMemoryUsed;
}

public class Job : IDisposable
{
    [DllImport("kernel32.dll", CharSet = CharSet.Unicode)]
    static extern IntPtr CreateJobObject(object a, string lpName);

    [DllImport("kernel32.dll")]
    static extern bool SetInformationJobObject(IntPtr hJob, JobObjectInfoType infoType, IntPtr lpJobObjectInfo, uint cbJobObjectInfoLength);

    [DllImport("kernel32.dll", SetLastError = true)]
    static extern bool AssignProcessToJobObject(IntPtr job, IntPtr process);

    private IntPtr m_handle;
    private bool m_disposed = false;

    public Job()
    {
        m_handle = CreateJobObject(null, null);

        JOBOBJECT_BASIC_LIMIT_INFORMATION info = new JOBOBJECT_BASIC_LIMIT_INFORMATION();
        info.LimitFlags = 0x2000;

        JOBOBJECT_EXTENDED_LIMIT_INFORMATION extendedInfo = new JOBOBJECT_EXTENDED_LIMIT_INFORMATION();
        extendedInfo.BasicLimitInformation = info;

        int length = Marshal.SizeOf(typeof(JOBOBJECT_EXTENDED_LIMIT_INFORMATION));
        IntPtr extendedInfoPtr = Marshal.AllocHGlobal(length);
        Marshal.StructureToPtr(extendedInfo, extendedInfoPtr, false);

        if (!SetInformationJobObject(m_handle, JobObjectInfoType.ExtendedLimitInformation, extendedInfoPtr, (uint)length))
            throw new Exception(string.Format("Unable to set information.  Error: {0}", Marshal.GetLastWin32Error()));
    }

    #region IDisposable Members

    public void Dispose()
    {
        Dispose(true);
        GC.SuppressFinalize(this);
    }

    #endregion

    private void Dispose(bool disposing)
    {
        if (m_disposed)
            return;

        if (disposing) {}

        Close();
        m_disposed = true;
    }

    public void Close()
    {
        Win32.CloseHandle(m_handle);
        m_handle = IntPtr.Zero;
    }

    public bool AddProcess(IntPtr handle)
    {
        return AssignProcessToJobObject(m_handle, handle);
    }

}

看着构造函数…

JOBOBJECT_BASIC_LIMIT_INFORMATION info = new JOBOBJECT_BASIC_LIMIT_INFORMATION();
info.LimitFlags = 0x2000;

这里的关键是正确设置作业对象。在构造函数中，我将“限制”设置为0x2000，这是的数字值JOB_OBJECT_LIMIT_KILL_ON_JOB_CLOSE。

MSDN将该标志定义为：

当作业的最后一个句柄关闭时，导致与该作业关联的所有进程终止。

设置好此类后，您只需在作业中注册每个子进程。例如：

[DllImport("user32.dll", SetLastError = true)]
public static extern uint GetWindowThreadProcessId(IntPtr hWnd, out uint lpdwProcessId);

Excel.Application app = new Excel.ApplicationClass();

uint pid = 0;
Win32.GetWindowThreadProcessId(new IntPtr(app.Hwnd), out pid);
 job.AddProcess(Process.GetProcessById((int)pid).Handle);